Being a teacher is indeed a calling, and not a carreer. I know a few teachers, and they do a very good job -- and I'm happy for that, because I couldn't do it.
I think he just looks incredulous. It's like, "Did you forget that I'm not just an actor but actually an incredibly smart and well-educated actor who will verbally kick your ass?"
I'll go with the incredulous and her realising he is stomping all over her (intellectually). All cred to her for staying shut up - many interviewers would not....
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I also like how he looks pissed off at her.
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I did like the, "...well maybe you're a shitty camera man?"